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Electrodeposition of a dendrite‐free 3D Al anode for improving cycling of an aluminum–graphite battery
Li, J.F.1; Hui, K.S.2; Ji, S.P.1; Zha, C.Y.1; Yuan, C.Z.1; Wu, S.X.3; Bin, F.4; Fan, X.5; Chen, Fuming6; Shao, Z.P.7,8; Hui, K.N.1
2022-03
Source PublicationCarbon Energy
Volume4Issue:2Pages:155
Abstract

Aluminum–metal batteries show great potential as next-generation energy storage due to their abundant resources and intrinsic safety. However, the crucial limitations of metallic Al anodes, such as dendrite and corrosion problems in conventional aluminum–metal batteries, remain challenging and elusive. Here, we report a novel electrodeposition strategy to prepare an optimized 3D Al anode on carbon cloth with an uniform deposition morphology, low local current density, and mitigatory volume change. The symmetrical cells with the 3D Al anode show superior stable cycling (>450 h) and low-voltage hysteresis (~170 mV) at 0.5 mA cm−2. High reversibility (~99.7%) is achieved for the Al plating/stripping. The graphite | | Al-4/CC full batteries show a long lifespan of 800 cycles with 54 mAh g−1 capacity at a high current density of 1000 mA g−1, benefiting from the high capacitive-controlled distribution. This study proposes a novel strategy to design 3D Al anodes for metallic-Al-based batteries by eliminating the problems of planar Al anodes and realizing the potential applications of aluminum–graphite batteries.

Keyword3d Al Anode, Ionic Liquid, metAllic, Plating/stripping, Stability
DOIdoi.org/10.1002/cey2.188
URLView the original
Indexed BySCIE
WOS Research AreaChemistry ; Energy & Fuels ; Science & Technology - Other Topics ; Materials Science
WOS SubjectChemistry, Physical ; Energy & Fuels ; Nanoscience & Nanotechnology ; Materials Science, Multidisciplinary
WOS IDWOS:000713345500001
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Cited Times [WOS]:3   [WOS Record]     [Related Records in WOS]
Document TypeJournal article
CollectionINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding AuthorHui, K.S.; Hui, K.N.
Affiliation1.Joint Key Laboratory of the Ministry of Education, Institute of Applied Physics and Materials Engineering, University of Macau, Avenida da Universidade, Taipa, Macau SAR, China
2.School of Engineering, Faculty of Science, University of East Anglia, Norwich, NR4 7TJ, United Kingdom
3.School of Chemical Engineering and Light Industry, Guangdong University of Technology, Guangzhou 510006, PR China
4.State Key Laboratory of High‐Temperature Gas Dynamics, Institute of Mechanics, Chinese Academy of Sciences, Beijing, China
5.Ningbo Institute of Materials Technology, Engineering, Chinese Academy of Sciences, Ningbo, 315201, PR China
6.Guangdong Provincial Key Laboratory of Quantum Engineering and Quantum Materials, School of Physics and Telecommunication Engineering, South China Normal University, 510006, PR China
7.State Key Laboratory of Organic-Inorganic Composites, Beijing University of Chemical Technology, 15 North Third Ring East Road, Chaoyang District, Beijing 100029 (P.R.China)
8.WA School of Mines: Minerals, Energy and Chemical Engineering (WASM-MECE), Curtin University, Perth, WA, 6102, Australia
First Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Corresponding Author AffilicationINSTITUTE OF APPLIED PHYSICS AND MATERIALS ENGINEERING
Recommended Citation
GB/T 7714
Li, J.F.,Hui, K.S.,Ji, S.P.,et al. Electrodeposition of a dendrite‐free 3D Al anode for improving cycling of an aluminum–graphite battery[J]. Carbon Energy,2022,4(2):155.
APA Li, J.F.,Hui, K.S.,Ji, S.P.,Zha, C.Y.,Yuan, C.Z.,Wu, S.X.,Bin, F.,Fan, X.,Chen, Fuming,Shao, Z.P.,&Hui, K.N..(2022).Electrodeposition of a dendrite‐free 3D Al anode for improving cycling of an aluminum–graphite battery.Carbon Energy,4(2),155.
MLA Li, J.F.,et al."Electrodeposition of a dendrite‐free 3D Al anode for improving cycling of an aluminum–graphite battery".Carbon Energy 4.2(2022):155.
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