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Persulfate-based controlled release beads for in situ chemical oxidation of common organic pollutants
Ma, Jie1; Ma, Yao1; Rong, Xun1; Song, Quanwei2,3; Wu, Baichun2,3; Lan, Xingying1; Feng, Yuan1; Qiu, Xiaoyuan4; Zhang, Ping4
2021-10-01
Source PublicationJournal of Environmental Chemical Engineering
ISSN2213-3437
Volume9Issue:5
Abstract

Groundwater contamination by organic pollutants is a growing threat to the environment and human health. As a cost-effective method, in situ chemical oxidation (ISCO) treatment has become a popular technical method to degrade groundwater pollutants. However, conventional ISCO treatment can suffer from a number of operational issues, such as tailing and concentration rebound, and thus the long-term treatment effectiveness is less desirable. As an alternative approach to the conventional ISCO method, controlled release materials are designated to gradually release oxidant chemicals to treat polluted groundwater with an extended chemical release duration and a reduced peak release rate. In this study, novel persulfate-paraffin based controlled release bead (CRB) materials were prepared and tested in a laboratory setting for their applicability in groundwater organic pollution remediation. It shows that bead size and temperature can substantially affect the release kinetics of persulfate from the CRBs, while the impact of solution pH and the presence of matrix anions are insignificant. Moreover, degradation experiments of benzene, toluene, ethylbenzene, and xylene pollutants show that the performance of CRBs, particularly within a short period after being delivered in situ, is on par with the conventional ISCO method using aqueous persulfate. This study expands our understanding and capacity in adopting controlled release materials for groundwater remediation. This study promotes the potential field application of such novel controlled release materials for environmental remediation of groundwater.

KeywordControlled Release Degradation Groundwater Isco Persulfate
DOI10.1016/j.jece.2021.105627
URLView the original
Indexed BySCIE
Language英語English
WOS Research AreaEngineering
WOS SubjectEngineering, Environmental ; Engineering, Chemical
WOS IDWOS:000703571000005
Scopus ID2-s2.0-85111140349
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Cited Times [WOS]:4   [WOS Record]     [Related Records in WOS]
Document TypeJournal article
CollectionDEPARTMENT OF CIVIL AND ENVIRONMENTAL ENGINEERING
Affiliation1.State Key Laboratory of Heavy Oil Processing, Beijing Key Lab of Oil & Gas Pollution Control, China University of Petroleum-Beijing, Beijing, 102249, China
2.State Key Laboratory of Petroleum Pollution Control, Beijing, 102206, China
3.CNPC Research Institute of Safety and Environmental Technology, Beijing, 102206, China
4.Department of Civil and Environmental Engineering, Faculty of Science and Technology, University of Macau, Taipa, Avenida da Universidade, Macao
Recommended Citation
GB/T 7714
Ma, Jie,Ma, Yao,Rong, Xun,et al. Persulfate-based controlled release beads for in situ chemical oxidation of common organic pollutants[J]. Journal of Environmental Chemical Engineering,2021,9(5).
APA Ma, Jie,Ma, Yao,Rong, Xun,Song, Quanwei,Wu, Baichun,Lan, Xingying,Feng, Yuan,Qiu, Xiaoyuan,&Zhang, Ping.(2021).Persulfate-based controlled release beads for in situ chemical oxidation of common organic pollutants.Journal of Environmental Chemical Engineering,9(5).
MLA Ma, Jie,et al."Persulfate-based controlled release beads for in situ chemical oxidation of common organic pollutants".Journal of Environmental Chemical Engineering 9.5(2021).
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